I had everything in my Dropbox: all my legal documents, my work-related files, my photos from the last 20 years, and things people sent me that I want to look at again when I'm 80… I literally had my life stored in it (and of course locally on two machines and a extra backup disk). I also accessed it almost daily via my phone and uploaded files from my phone.
So, I tested several services in the range of ~100 Euros a year with at least 1,5 Terabytes:
Jottacloud:
Good Desktop Client (Win & Mac)
Very good iOS App
Good service
Pricey (144 Euros for unlimited storage)
Downside for me: it doesn't automatically convert photo uploads from my phone to JPG and doesn't store them in a folder I choose – plus, the price is high.
Filen:
Good Desktop Client (Win & Mac)
Rough iOS App
Good service
Okay price (108 Euros for 2TB)
Downside for me: the rough iOS App didn't have a document upload with a scan function.
Nextcloud:
Good Desktop Client (Win & Mac)
Good iOS App
No dedicated service; it's Open Source, so some tinkering is required since you manage the hosting yourself.
Weird price range (Hetzner, the cheapest host by far, offers either 60 Euros for 1TB or 200 Euros for 5TB, nothing in between).
Downside for me: the price range.
kDrive:
Good Desktop Client (Win & Mac)
Very good iOS App
Amazing service, document editing included, etc.
Amazing price (60 Euros per year for 3TB)
Downside for me: none.
So, I chose kDrive, even though I'd love to use Nextcloud because it's Open Source and you can choose your own host. If I needed less than 1TB, I'd definitely choose Nextcloud.
And it should be said that all the services I tested offer free options with a few Gigabytes, if that's all you need.